个人简述:
吕汪洋,男,工学博士,副教授,硕士生导师,入选浙江省151人才工程和校521人才工程。攻读博士学位期间主要从事纤维材料的催化功能化研究,博士论文“催化功能纤维降解染料等有机污染的研究”获2010年浙江省优秀博士学位论文,并获得2012年全国优秀博士学位论文提名论文,主持国家自然科学基金项目一项,参与国家自然科学基金重点项目一项(排名第二),主持浙江省自然科学基金项目两项、浙江省科技厅项目两项,主持或参与完成包括国家自然科学基金、教育部“新世纪优秀人才支持计划”项目在内的十多项国家和省部级科研项目,先后在国内外重要学术刊物如:《Environ. Sci. Technol.》、《Appl. Catal. B: Environ.》、《Carbon》、《Cellulose》、《React. Funct. Polym.》和《Sci. China Chem.》等发表学术论文60余篇,其中SCI、EI论文40余篇,申请国家发明专利15项,授权10项。以第二完成人获浙江省科学技术奖一等奖和中国纺织工业协会科技进步奖一等奖各1项。
科研工作:
近期代表性论文
[1]Chen, X.,Lu, W.,* Xu, T., Li, N., Qin, D., Zhu, Z., Wang, G., Chen, W.* A bio-inspired strategy to enhance the photocatalytic performance of g-C3N4 under solar irradiation by axial coordination with hemin.(2017) Applied Catalysis B: Environmental, 201, pp. 518-526.
[2]Qin, D.,Lu, W.,* Wang, X., Li, N., Chen, X., Zhu, Z., Chen, W.* Graphitic carbon nitride from burial to re-emergence on polyethylene terephthalate nanofibers as an easily recycled photocatalyst for degrading antibiotics under solar irradiation. (2016) ACS Applied Materials & Interfaces, Article in Press.
[3]Xu, T., Ni, D., Chen, X., Wu, F., Ge, P.,Lu, W.,* Hu, H., Zhu, Z., Chen, W.* Self-floating graphitic carbon nitride/zinc phthalocyanine nanofibers for photocatalytic degradation of contaminants.(2016) Journal of Hazardous Materials, 317, pp. 17-26.
[4]Chen, S., Zhang, X., Liu, M., Ma, J.,Lu, W.,Chen, W.* Rheological characterization and thermal stability of different intrinsic viscosity poly(ethylene terephthalate) in air and nitrogen.(2016) International Polymer Processing, 31 (3), pp. 292-300.
[5]Zhu, Z., Chen, Y., Gu, Y., Wu, F.,Lu, W.,* Xu, T., Chen, W.* Catalytic degradation of recalcitrant pollutants by Fenton-like process using polyacrylonitrile-supported iron (II) phthalocyanine nanofibers: Intermediates and pathway.(2016) Water Research, 93, pp. 296-305.
[6]Hu, J., Liu, H., Wang, L., Li, N., Xu, T.,Lu, W.,* Zhu, Z., Chen, W.* Electronic properties of carbon nanotubes linked covalently with iron phthalocyanine to determine the formation of high-valent iron intermediates or hydroxyl radicals. (2016) Carbon, 100, pp. 408-416.
[7]Liu, M., Xia, H.,Lu, W.,* Xu, T., Zhu, Z., Chen, W.* Electrocatalytic degradation of organic contaminants using carbon fiber coupled with cobalt phthalocyanine electrode.(2016) Journal of Applied Electrochemistry, 46, pp. 583-592.
[8]Lu, W.,* Xu, T., Wang, Y., Hu, H., Li, N., Jiang, X., Chen, W.* Synergistic photocatalytic properties and mechanism of g-C3N4 coupled with zinc phthalocyanine catalyst under visible light irradiation. (2016) Applied Catalysis B: Environmental, 180, pp. 20-28.(ESI高被引论文)
[9]Li, N.,Lu, W.,* Pei, K., Chen, W.* Interfacial peroxidase-like catalytic activity of surface-immobilized cobalt phthalocyanine on multiwall carbon nanotubes.(2015) RSC Advances, 5 (13), pp. 9374-9380.
[10]Li, N.,Lu, W.,* Pei, K., Yao, Y., Chen, W.* Formation of high-valent cobalt-oxo phthalocyanine species in a cellulose matrix for eliminating organic pollutants. (2015) Applied Catalysis B: Environmental, 163, pp. 105-112.被引用6次.
[11]Xu, T., Wu, F., Gu, Y., Chen, Y., Cai, J.,Lu, W.,* Hu, H., Zhu, Z., Chen, W.* Visible-light responsive electrospun nanofibers based on polyacrylonitrile-dispersed graphitic carbon nitride. (2015) RSC Advances, 5 (105), pp. 86505-86512.
[12]Li, N.,Lu, W.,* Pei, K., Yao, Y., Chen, W.* Ordered-mesoporous-carbon-bonded cobalt phthalocyanine: A bioinspired catalytic system for controllable hydrogen peroxide activation. (2014) ACS Applied Materials and Interfaces, 6 (8), pp. 5869-5876.被引用7次.
[13]Gao, M., Li, N.,Lu, W.,* Chen, W.* Role of cellulose fibers in enhancing photosensitized oxidation of basic green 1 with massive dyeing auxiliaries. (2014) Applied Catalysis B: Environmental, 147, pp. 805-812.被引用6次.
[14]Gao, M.,Lu, W.,* Li, N., Chen, W.* Enhanced removal of acid red 1 with large amounts of dyeing auxiliaries: The pivotal role of cellulose support. (2014) Cellulose, 21 (3), pp. 2073-2087.
[15]Chen, S.,Lu, W.,* Yao, Y., Chen, H., Chen, W. Oxidative desulfurization of dibenzothiophene with molecular oxygen catalyzed by carbon fibersupported iron phthalocyanine. (2014) Reaction Kinetics, Mechanisms and Catalysis, 111 (2), pp. 535-547.
[16]Lu, W.,* Sun, C., Lu, Q., Li, N., Wu, D., Yao, Y., Chen, W.* Synthesis and photoactivity of pH-responsive amphiphilic block polymer photosensitizer bonded zinc phthalocyanine. (2012) Science China Chemistry, 55 (6), pp. 1108-1114.
[17]Lu, W.,Li, N., Bao, S., Chen, W.,* Yao, Y. The coupling of metallophthalocyanine with carbon nanotubes to produce a nanomaterial-based catalyst for reaction-controlled interfacial catalysis. (2011) Carbon, 49 (5), pp. 1699-1709.被引用12次.
[18]Chen, W.,*Lu, W.,Shen, X., Yao, Y. Photocatalytic oxidation of 4-chlorophenol using thermosensitive zinc phthalocyanine copolymer under visible light irradiation. (2010) Science China Chemistry, 53 (3), pp. 638-644.被引用7次.
[19]Lu, W.,Zhao, B., Li, N., Yao, Y., Chen, W.* Thermosensitive copolymer with cobalt phthalocyanine and catalytic behavior based on adjustable LCST. (2010) Reactive and Functional Polymers, 70 (3), pp. 135-141.被引用9次.
[20]Lu, W.,Li, N., Chen, W.,* Yao, Y. The role of multiwalled carbon nanotubes in enhancing the catalytic activity of cobalt tetraaminophthalocyanine for oxidation of conjugated dyes. (2009) Carbon, 47 (14), pp. 3337-3345.被引用41次.
[21]Lu, W.,Chen, W.,* Li, N., Xu, M., Yao, Y. Oxidative removal of 4-nitrophenol using activated carbon fiber and hydrogen peroxide to enhance reactivity of metallophthalocyanine. (2009) Applied Catalysis B: Environmental, 87 (3-4), pp. 146-151.被引用42次.
[22]Shen, X.,Lu, W.,Feng, G., Yao, Y., Chen, W.* Preparation and photoactivity of a novel water-soluble, polymerizable zinc phthalocyanine. (2009) Journal of Molecular Catalysis A: Chemical, 298 (1-2), pp. 17-22.被引用12次.
[23]Chen, W.,* Liu, F.,Lu, W.,Shen, X., Yao, Y., Xu, M. Preparation and photoactivity of thermosensitive polymer supported metallophthalocyanine. (2008) Science in China, Series B: Chemistry, 51 (6), pp. 570-576.
[24]Feng, G., Shen, X., Li, N., Zhao, B., Yao, Y.,Lu, W.,Chen, W.* Preparation and properties of a novel thermosensitive polymer containing cobalt phthalocyanine. (2008) Acta Polymerica Sinica, (6), pp. 567-573.
[25]Chen, W.,*Lu, W.,Yao, Y., Xu, M. Highly efficient decomposition of organic dyes by aqueous-fiber phase transfer and in situ catalytic oxidation using fiber-supported cobalt phthalocyanine. (2007) Environmental Science and Technology, 41 (17), pp. 6240-6245.被引用111次.
[26]Gong, F., Luo, L., Yao, Y., Dai, D.,Lu, W.,Chen, W. Drastic rate acceleration driven by synergistic effects: Key role of persistent free radicals coupled with ascorbic acid in decomposition of organic contaminants by ferric citrate.(2016) Chemical Engineering Journal, 304, pp. 440-447.
[27]Huang, Z., Bao, H., Yao, Y., Lu, J.,Lu, W.,Chen, W. Key role of activated carbon fibers in enhanced decomposition of pollutants using heterogeneous cobalt/peroxymonosulfate system.(2016) Journal of Chemical Technology and Biotechnology, 91 (5), pp. 1257-1265.被引用2次.
[28]Jiang, B., Yao, Y., Xie, R., Dai, D.,Lu, W.,Chen, W., Zhang, L.Enhanced generation of reactive oxygen species for efficient pollutant elimination catalyzed by hemin based on persistent free radicals.(2016) Applied Catalysis B: Environmental, 183, pp. 291-297.
[29]Zhuang, Y., Lin, Q., Zhang, L., Luo, L., Yao, Y.,Lu, W.,Chen, W. Mesoporous carbon-supported cobalt catalyst for selective oxidation of toluene and degradation of water contaminants.(2016) Particuology, 24, pp. 216-222.
[30]Huang, Z., Yao, Y., Lu, J., Chen, C.,Lu, W.,Huang, S., Chen, W. The consortium of heterogeneous cobalt phthalocyanine catalyst and bicarbonate ion as a novel platform for contaminants elimination based on peroxymonosulfate activation.(2016) Journal of Hazardous Materials, 301, pp. 214-221.
[31]Luo, L., Yao, Y., Gong, F., Huang, Z.,Lu, W.,Chen, W., Zhang, L. Drastic enhancement on Fenton oxidation of organic contaminants by accelerating Fe(III)/Fe(II) cycle with l-cysteine.(2016) RSC Advances, 6 (53), pp. 47661-47668.
[32]Zhou, F., Lu, C., Yao, Y., Sun, L., Gong, F., Li, D., Pei, K.,Lu, W.,Chen, W. Activated carbon fibers as an effective metal-free catalyst for peracetic acid activation: Implications for the removal of organic pollutants.(2015) Chemical Engineering Journal, 281, pp. 953-960.
[33]Gong, F., Wang, L., Li, D., Zhou, F., Yao, Y.,Lu, W.,Huang, S., Chen, W. An effective heterogeneous iron-based catalyst to activate peroxymonosulfate for organic contaminants removal.(2015) Chemical Engineering Journal, 267, pp. 102-110.
[34]Huang, Z., Ye, Y., Zhu, S., Yao, Y.,Lu, W.,Chen, W. Enhanced catalytic decoloration of Rhodamine B based on 4-aminopyridine iron coupled with cellulose fibers. (2015) Journal of Chemical Technology and Biotechnology, 90 (6), pp. 1144-1151.
[35]Wang, L., Yao, Y., Zhang, Z., Sun, L.,Lu, W.,Chen, W., Chen, H. Activated carbon fibers as an excellent partner of Fenton catalyst for dyes decolorization by combination of adsorption and oxidation. (2014) Chemical Engineering Journal, 251, pp. 348-354.
[36]Huang, Z., Ye, Y., Zhu, S., Yao, Y.,Lu, W.,Chen, W. Enhanced catalytic decoloration of Rhodamine B based on 4-aminopyridine iron coupled with cellulose fibers. (2014) Journal of Chemical Technology and Biotechnology, . Article in Press.
[37]Huang, Z., Bao, H., Yao, Y.,Lu, W.,Chen, W. Novel green activation processes and mechanism of peroxymonosulfate based on supported cobalt phthalocyanine catalyst. (2014) Applied Catalysis B: Environmental, 154-155, pp. 36-43.被引用33次.
[38]Yao, Y., Mao, Y., Zheng, B., Huang, Z.,Lu, W.,Chen, W. Anchored iron ligands as an efficient fenton-like catalyst for removal of dye pollutants at neutral pH. (2014) Industrial and Engineering Chemistry Research, 53 (20), pp. 8376-8384.被引用5次.
[39]Sun, L., Yao, Y., Wang, L., Mao, Y., Huang, Z., Yao, D.,Lu, W.,Chen, W. Efficient removal of dyes using activated carbon fibers coupled with 8-hydroxyquinoline ferric as a reusable Fenton-like catalyst. (2014) Chemical Engineering Journal, 240, pp. 413-419.
[40]Wang, L., Yao, Y., Sun, L., Mao, Y.,Lu, W.,Huang, S., Chen, W. Rapid removal of dyes under visible irradiation over activated carbon fibers supported Fe(III)-citrate at neutral pH. (2014) Separation and Purification Technology, 122, pp. 449-455.
[41]Yao, Y., Mao, Y., Huang, Q., Wang, L., Huang, Z.,Lu, W.,Chen, W. Enhanced decomposition of dyes by hemin-ACF with significant improvement in pH tolerance and stability. (2014) Journal of Hazardous Materials, 264, pp. 323-331.
[42]Huang, Z., Zheng, B., Zhu, S., Yao, Y., Ye, Y.,Lu, W.,Chen, W. Photocatalytic activity of phthalocyanine-sensitized TiO 2-SiO2 microparticles irradiated by visible light. (2014) Materials Science in Semiconductor Processing, 25, pp. 148-152.
[43]Wang, L., Yao, Y., Sun, L.,Lu, W.,Chen, W. Activation of hydrogen peroxide by activated carbon fibers coupled with Fe(III)-citrate for degradation of dyes at Neutral pH. (2013) Acta Chimica Sinica, 71 (12), pp. 1633-1638.
[44]Yao, Y., Huang, Z., Zheng, B., Zhu, S.,Lu, W.,Chen, W., Chen, H. Photocatalytic degradation of dyes using dioxygen activated by supported metallophthalocyanine under visible light irradiation. (2013) Current Applied Physics, 13 (8), pp. 1738-1742.
[45]Yao, Y., Jiang, C.,Lu, W.,Liu, H., Wang, X., Chen, W. Synthesis and crytallization properties of cationic dyeable poly (trimethylene terephthalate) copolyesters. (2011) Acta Polymerica Sinica, (5), pp. 467-474.
授权专利:
[1]吕汪洋,陈文兴,姚玉元.一种检测过氧化氢浓度的试剂及方法.中国发明专利,专利号: 200910099059.X.
[2]吕汪洋,李楠,吕巧莉,陈文兴,姚玉元.一种双活性反应型环糊精及制备方法.中国发明专利,专利号: 201110256684.8.
[3]陈文兴,吕汪洋,徐敏虹,姚玉元.一种有机废水的处理方法.中国发明专利,专利号: 200810059241.8.
[4]陈文兴,姚玉元,吕汪洋.抗静电、导电和电磁屏蔽纺织品及其制备方法.专利号:200910099533.9.
[5]陈文兴,姚玉元,吕汪洋.一种导电纤维及其制备方法.专利号:200910099534.3.
[6]陈文兴,陈辉,姚玉元,吕汪洋.一种聚酰亚胺纤维及其制备方法.专利号: 201110256670.6
获奖情况:
[1]吕汪洋.博士论文《催化功能纤维降解染料等有机污染的研究》获全国优秀博士学位论文提名奖,2012.
[2]陈文兴,吕汪洋,姚玉元,王晟,王騊,李楠.环境催化纤维的设计制备及降解有机污染物的研究,浙江省人民政府,浙江省科学技术奖,一等奖, 2011.
[3]陈文兴,吕汪洋,姚玉元,王晟,胡智文,王騊,李楠.催化功能性纤维及其应用基础研究,中国纺织工业协会,中国纺织工业协会科学技术奖,一等奖, 2011.
[4]陈文兴,吕汪洋,姚玉元,徐敏虹.基于纤维键合酞菁催化剂的"相转移原位催化氧化技术"及其高效降解染料的研究.浙江省自然科学学术奖,一等奖, 2010.
科研项目:
[1]国家自然科学基金项目:可见光响应催化纤维选择性消除染料等有机污染物(主持)
[2]国家自然科学基金重点项目:环境催化纤维多场驱动下消除有机污染物的研究(参与,排名第二)
[3]国家973计划前期研究专项:高效能熔融缩聚制备高黏聚酯熔体的基础研究(参与,排名第三)
[4]中国纺织工业联合会应用基础研究项目:环境催化纤维降解染料的基础研究(主持)
[5]浙江省自然科学基金项目:新型催化功能纤维的构筑及选择性消除持久性有机污染物(主持)
[6]浙江省自然科学基金项目:活性碳与金属酞菁协同催化降解典型持久性有机污染物的研究(主持)
[7]浙江省科技厅一般项目:纤维接枝包络维生素E的研究(主持)
[8]浙江省科技厅一般项目:新型聚酰亚胺的制备及其可纺性研究(主持)
[9]企业委托项目:非金属材料一致性鉴定分析技术研究(主持)